Okay, while I love the amount of expressions you've given him here, especially the one with a frontal view which we don't get often from the show, I have to laugh at how you made the aura from his eyes burst forth like steam when he gets angry! Brilliant!
the head-on one that's not the smoke cloud should be when he says "GRRRRRR! THAT IS MINE!" and when he growls before saying "that is mine" the smoke should already be there and shoot up vertical (and by "already be there " I mean as in EVERY SCENE OF him should have that eyesmoke and green sclera (the official name fore the white part of your eyes)present, just the length and direction of the eyesmoke would change (but it would never point forward))
Thanks man! XD The one with smoke from his eyes is my personal fav; I can imagine him growing bigger, covering himself with the dark fog, kinda like Ursula does in the last final battle in The Little Mermaid